One anime that really stands out with its unique storytelling is "KonoSuba: God's Blessing on This Wonderful World!" While it might not be underrated per se, it plays with the conventions of the isekai genre in such a self-aware way that it feels fresh. The characters constantly break the fourth wall, and the humor often subverts the typical heroic tropes you find in similar series.
Another hidden gem to check out is "The Tatami Galaxy." The non-linear storytelling and the way it explores different timelines and choices is nothing short of brilliant. Masaaki Yuasa's distinct animation style complements its themes of youth and regret perfectly. It's a wild ride that can leave you pondering long after it's over.
If you're looking for something truly experimental, "Kaiba" might be worth a look. It has such a unique aesthetic and narrative structure that plays with memory, identity, and even the concept of love in a very unconventional way.
What kind of themes or genres are you more interested in? I'd love to recommend more specific titles based on that!