Super Sentai Suits

But could they just kind of...Walk around in them if they wanted?

In addition to that Changeman episode Shougo mentioned, there's a Goseiger episode that offers a much goofier take on this scenario. It's episode 4, I believe.

In most shows, the characters won't just hang around in-suit to make the suits seem more special. The big exception I can think of offhand is Fourze, where Gentaro is perfectly capable of just chillin' in the Fourze suit.
 
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